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/content/aip/journal/adva/1/4/10.1063/1.3666981
2011-11-29
2016-12-05

Abstract

We demonstrated an efficient sequential two-step near-infrared (NIR) quantum splitting (QS) in a Ho3+ singly dopedβ-NaYF4. An incident high-energy ultraviolet (UV)-to-visible photon in the wavelength range of 300−560 nm, which enables the Ho3+:5F4,5S2 states excited, could be efficiently split into two NIR photons at 1015 and 1180 nm. Underlying mechanisms for the sequential two-step NIR-QS process are analyzed in terms of the diffuse reflection spectrum, static and dynamic photoemissionspectra and monitored excitation spectra. Internal quantum yield is obtained up to 110% on the basis of experimental and theoretical calculation results.

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