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Enhanced three-photon near-infrared quantum splitting in β-NaYF4:Ho3+ by codoping Yb3+
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/content/aip/journal/adva/2/2/10.1063/1.4718412
2012-05-08
2014-07-24

Abstract

An efficient three-step sequential three-photon near-infrared (NIR) quantum splitting (QS), involving the emission of three NIR photons from an absorbed ultraviolet (UV)photon in β-NaYF4:Ho3+, has been demonstrated. Codoping Yb3+ can increase the NIR emissions significantly through the first- and second-step cross-relaxation. The involved mechanisms of three-step NIR QS in Ho3+-Yb3+ have been well demonstrated by the static and dynamic photoluminescence, monitored excitation and time-resolved fluorescencespectra. An internal quantum yield (QY) of 246% for the Yb3+ codoped β-NaYF4:Ho3+ is estimated on the basis of experimental data and theoretical considerations, which is much more than the total QY of 124% for the β-NaYF4:Ho3+ three-photon NIR QS. This research may open up promising new perspectives for designing efficient photonic devices.

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Scitation: Enhanced three-photon near-infrared quantum splitting in β-NaYF4:Ho3+ by codoping Yb3+
http://aip.metastore.ingenta.com/content/aip/journal/adva/2/2/10.1063/1.4718412
10.1063/1.4718412
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