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/content/aip/journal/adva/5/11/10.1063/1.4935340
2015-11-03
2016-12-05

Abstract

The fragmentation dynamics of CH and HCO molecules have been studied with ultra-short pulses at laser intensityof up to 1015Wcm−2. Three dimensional molecular dynamics calculations for finding the optimized laser pulses are presented based on time-dependent density functional theory and quantum optimal control theory. A comparison of the results for orientation dependence in the ionization process shows that the electron distribution for CH is more isotropic than HCO molecule. Total conversion yields of up to 70% at an orientation angle of 30o for CH and 65% at 900 for HCO are achieved which lead to enhancement of dissociation probability.

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