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/content/aip/journal/adva/6/2/10.1063/1.4942753
2016-02-22
2016-09-27

Abstract

We report structural, optical, and electro-optical properties of polycrystalline YFeOthin films,deposited on (0001) sapphire substrates using the electron-beam deposition technique. The optical spectra of a 120 nm YFeO show Fe to on-site and O 2 to Fe 3, Y 4, and Y 5charge-transfer electronic excitations. Anomalies in the temperature dependence data of the charge-transfer excitations and the splitting of the 4.46 eV charge-transfer peak strongly suggest a structural distortion at 180 ± 10 K. Evidence of such a structural distortion is also manifested in the surface resistance versus temperature data. In addition, the YFeOthin film at low temperatures shows strong electro-optical properties, as high as 9% in the energy range of 1 - 2.5 eV, for applied electric fields up to 500 V.cm−1.

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