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A polymer electrolyte with high luminous transmittance and low solar throughput: Polyethyleneimine-lithium bis(trifluoromethylsulfonyl) imide with In2O3:Sn nanocrystals
2. G. B. Smith and C. G. Granqvist, Green Nanotechnology: Solutions for Sustainability and Energy in the Built Environment (CRC, Boca Raton, FL, 2010).
4. C. G. Granqvist, Handbook of Inorganic Electrochromic Materials (Elsevier, Amsterdam, The Netherlands, 1995).
10.Recently, compositional tuning of the near-infrared plasmon absorption was demonstrated for solvent-dispersed ITO nanocrystals synthesized by organic phase colloidal methods; cf. M. Kanehara, H. Koike, T. Yoshinaga, and T. Teranishi, J. Am. Chem. Soc. 131, 17736 (2009)
10.and G. Garcia, R. Buonsanti, E. L. Runnerstrom, R. J. Mendelsberg, A. Llordes, A. Anders, T. J. Richardson, and D. J. Milliron, Nano Lett. 11, 4415 (2011).
14. G. Wyszecki and W. S. Stiles, Color Science: Concepts and Methods, Quantitative Data and Formulae, 2nd ed. (Wiley, New York, 2000).
ASTM G173-03 Standard Tables of Reference Solar Spectral Irradiances: Direct Normal and Hemispherical on a 37° Tilted Surface, Annual Book of ASTM Standards
(American Society for Testing and Materials
, Philadelphia, PA
), Vol. 14.04; http://rredc.nrel.gov/solar/spectra/am1.5
22.Refractive index was taken from published data for PEI [ T. M. Madkour, in Polymer Data Handbook, edited by J. E. Mark (Oxford University Press, Oxford, UK, 1999), pp. 490–492]; absorption coefficient was determined from the ratio of the transmittance of the polymer between the glass slides to the transmittance of the bare glass slides without spacer.
23.The random phase approximation [ J. Lindhard, Kgl. Danske Videnskab. Selskab Mat.-Fys. Medd. 28(8) (1954)] was corrected for exchange
23.is possible but is not expected to be significant. In principle, ɛITO should be corrected for a limited mean free path ℓ of the free electrons caused by the small particle size [ U. Kreibig and M. Vollmer, Optical Properties of Metal Clusters (Springer, Berlin, Germany, 1995)], but this effect is believed to be minor since ℓ is as short as ∼5 nm in the infrared (though increasing progressively towards shorter wavelengths since screening of the tin ions then becomes less efficient).
25. P. Clippe, R. Evrard, and A. A. Lucas, Phys. Rev. B 14, 1715 (1976).
25.Their approach relied on detailed calculations on the resonance frequencies for several geometrically well-defined entities comprised of identical spheres such as pairs, infinite single- and double strand chains, and a close-packed fcc lattice. It was used in earlier work on gas evaporated gold (Ref. 18), which is a three-dimensional composite of metal and air. In principle, higher order multipole effects might be needed in a more complete analysis [ A. Pack, M. Hietschold, and R. Wannemacher, Opt. Commun. 194, 277 (2001)],
25.but their effect is small since our ITO nanocrystals are separated from each other as inferred from recent work on samples similar to those studied in this Letter [ R. J. Mengelsberg, G. Garcia, and D. J. Milliron, J. Appl. Phys. 111, 063515 (2012)].
27. Polymer Electrolytes: Fundamentals and Applications, edited by C. Sequeira and D. Santos (Woodhead, Sawston, UK, 2010).
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