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/content/aip/journal/apl/107/7/10.1063/1.4928758
2015-08-17
2016-10-01

Abstract

Carrier recombination is a central process in bulk heterojunction organic solar cells. Based on the competition of hopping rates that either implies escape in a broad density of states or recombination across the interface, we formulate a general theory of recombination flux that distinguishes reaction or transport limited recombination according to charge density. The Langevin picture is valid only in the low charge density limit, and a crossover to the reaction controlled regime occurs at higher densities. We present results from impedance spectroscopy of poly(3-hexylthiophene):methanofullerene solar cell that exhibit this crossover.

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