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Experimental evidence of laser‐induced separations in bulk gas mixtures
1.A. Ashkin, Phys. Rev. Lett. 24, 156 (1970).
2.J. Gelbwachs and T. S. Hartwick, IEEE J. Quantum Electron. QE‐11, 52 (1975).
3.E. A. Rinehart, J. H. Richardson, and L. W. Hrubesh, University of California, LLL Report No. UCRL‐51833, 1975 (unpublished).
4.R. E. Dickerson, Molecular Thermodynamics (Benjamin, New York, 1969).
5.The derivation is similar to that of the thermodynamics of an isothermal atmosphere [F. T. Wall, Chemical Thermodynamics (Freeman, San Francisco, 1965)]. The salient difference is that the laser force field cannot support a large pressure gradient and that all the components do not experience the force field; it is thus apparent that the experiment is also similar to osmosis.
6.The experimental uncertainty (precision) was established over several days and included all random measurement errors (sampling, surface adsorption, spectrometer instability, etc.).
7.M. C. Mercy, D. Silhouette, and J. Conrad, C. R. Acad. Sci. Paris B 275, 693 (1972).
8.J. O. Hershfelder, C. F. Curtiss, and R. B. Bird, Molecular Theory of Gases and Liquids (Wiley, New York, 1964).
9.This is intuitively reasonable and is consistent with the longer times reported for velocity thermalization: P. R. Berman, J. M. Levy, and R. G. Brewer, Phys. Rev. A 11, 1668 (1975).
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