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Off‐resonant third‐order optical nonlinearities of metal‐substituted phthalocyanines
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8.An earlier report of degenerate four‐wave mixing experiments on the metal‐free, Cu, and Ni tetrakis(cumylphenoxy)‐phthalocyanines did not show a strong metal dependence [P. N. Prasad, M. K. Casstevens, J. Pfleger, and P. Legation, Proc. SPIE 878, 106 (1988)]. However, these measurements were at 605 nm in the absorption hand. The observed was ascribed to saturable absorption of the Q band, a different mechanism from the susceptibility at 1.064 μm.
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