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Interferometric differentiation between resonant coherent anti-Stokes Raman scattering and nonresonant four-wave-mixing processes
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10.1063/1.1829162
/content/aip/journal/apl/85/23/10.1063/1.1829162
http://aip.metastore.ingenta.com/content/aip/journal/apl/85/23/10.1063/1.1829162
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

A simulation of the pulse combination used to differentiate between resonant and nonresonant signals. The pump∕Stokes combination overlap to excite CARS, and the anti-Stokes would appear similar to the shown wave form for resonant or nonresonant media.

Image of FIG. 2.
FIG. 2.

Schematic of optical setup used to measure the interferogram of resonant and nonresonant signals.

Image of FIG. 3.
FIG. 3.

Partial Raman spectrum of acetone (upper left), and the cross-correlation interferogram of four-wave mixing in acetone at various vibrational excitation frequencies (a)–(c).

Image of FIG. 4.
FIG. 4.

Interferogram of nonresonant four-wave mixing in water (inset), and the power of the resonant anti-Stokes signal for various percentages of acetone in water by volume.

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/content/aip/journal/apl/85/23/10.1063/1.1829162
2004-12-08
2014-04-25
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Interferometric differentiation between resonant coherent anti-Stokes Raman scattering and nonresonant four-wave-mixing processes
http://aip.metastore.ingenta.com/content/aip/journal/apl/85/23/10.1063/1.1829162
10.1063/1.1829162
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