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Femtosecond investigation of the non-instantaneous third-order nonlinear suceptibility in liquids and glasses
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10.1063/1.2136413
/content/aip/journal/apl/87/21/10.1063/1.2136413
http://aip.metastore.ingenta.com/content/aip/journal/apl/87/21/10.1063/1.2136413

Figures

Image of FIG. 1.
FIG. 1.

Transient transmission change measured in (a) and (c) for parallel (dashed line) and perpendicular (full line) pump-probe polarizations. The pulse duration is about 100 fs (a) and 15 fs (c). Dependence on the average pump power of the peak to peak transmission change amplitude in (b) and (d) for parallel (squares) and perpendicular (dots) pump-probe polarizations. The ratios of the slopes of the linear fits yield in and in .

Image of FIG. 2.
FIG. 2.

Average pump power dependence of the peak to peak transmission change, , measured with 100 fs pulses in SF6 for parallel (squares) and perpendicular (dots) pump-probe polarizations. The ratio of the slopes of the linear fits yields . The inset shows the transient transmission change measured for parallel (dashed line) and perpendicular (full line) pump-probe polarizations for a pump power of 260 mW.

Image of FIG. 3.
FIG. 3.

Measured ratio as a function of the pulse duration in (full dots) and SF6 (full triangles) glasses. The dotted lines are guides to the eye.

Tables

Generic image for table
Table I.

Ratio, , obtained from the time-domain data in different liquids using 100 fs pulses.

Generic image for table
Table II.

Lead oxide (PbO) molar concentration of the SF glasses, ratio measured in time-domain experiments with 100 fs, precision of these measurements, and values obtained by Hellwarth using a spectral technique (Ref. 5), in silica and SF glasses.

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/content/aip/journal/apl/87/21/10.1063/1.2136413
2005-11-18
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Femtosecond investigation of the non-instantaneous third-order nonlinear suceptibility in liquids and glasses
http://aip.metastore.ingenta.com/content/aip/journal/apl/87/21/10.1063/1.2136413
10.1063/1.2136413
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