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Modified triphenylmethane dye for the efficient nonlinear generation of light in nanostructured materials
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10.1063/1.2773934
/content/aip/journal/apl/91/8/10.1063/1.2773934
http://aip.metastore.ingenta.com/content/aip/journal/apl/91/8/10.1063/1.2773934
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Chemical structure of (a) malachite green, (b) the derivative of the triphenylmethane with a triple bond (tH), and (c) with a double bond (dH).

Image of FIG. 2.
FIG. 2.

(Color online) Polar coordinate representation of the linear polarized SH intensity ( axis) as a function of the fundamental linear polarization ( axis) from (a) the bare prism interface, (b) the MG monolayer, and (c) the tH monolayer. TE (solid circles: experiment and solid line: theory) and TM (solid squares: experiment and dotted line: theory) SH intensities. Both theoretical and experimental values were normalized to the maximum generation obtained from the bare prism interface.

Image of FIG. 3.
FIG. 3.

(Color online) Absorption spectrum of the MG (dotted line), the dH homolog (dashed line), and the tH homolog (solid line). The indicates the molar absorption at for each chromophore.

Image of FIG. 4.
FIG. 4.

(Color online) Predicted total SH intensity as a function of the size of the crystal when the molecule is MG (dotted line, left axis), or dH (solid line, left axis), or tH (dashed line, right axis) for a TE fundamental incident at 45°. Normalization is to the maximum intensity of the MG. In the inset is a zoom of the first .

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/content/aip/journal/apl/91/8/10.1063/1.2773934
2007-08-23
2014-04-25
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Modified triphenylmethane dye for the efficient nonlinear generation of light in nanostructured materials
http://aip.metastore.ingenta.com/content/aip/journal/apl/91/8/10.1063/1.2773934
10.1063/1.2773934
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