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An x-ray probe of laser-aligned molecules
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10.1063/1.2890846
/content/aip/journal/apl/92/9/10.1063/1.2890846
http://aip.metastore.ingenta.com/content/aip/journal/apl/92/9/10.1063/1.2890846
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Schematic of experimental setup, top view. Inset with projection of interaction region: jet, collimation slit geometry, and Si drift detectors (D).

Image of FIG. 2.
FIG. 2.

X-ray absorption spectrum of near the -edge. Experimental data (dots). The Br resonance of at is marked with a vertical line. The fitted components and their sum are shown: Br resonance (dash dot), -edge (dashed), and sum (solid).

Image of FIG. 3.
FIG. 3.

(a) Laser/x-ray cross correlation for laser-aligned , ∥/⊥ absorption as a function of laser/x-ray delay. Theory for a rotational temperature is overlaid. (b) Calculated for a (FWHM) laser pulse with an intensity of for .

Image of FIG. 4.
FIG. 4.

Laser-on/laser-off ratio of Br fluorescence induced by x-ray excitation on the Br resonance of at , as a function of . and 90° correspond to the parallel and perpendicular configurations for laser and x-ray polarizations. Theory for is the overlaid curve.

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/content/aip/journal/apl/92/9/10.1063/1.2890846
2008-03-06
2014-04-19
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: An x-ray probe of laser-aligned molecules
http://aip.metastore.ingenta.com/content/aip/journal/apl/92/9/10.1063/1.2890846
10.1063/1.2890846
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