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Regioregular poly(3-hexyl-thiophene) helical self-organization on carbon nanotubes
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Mixtures of regioregular poly(3-hexyl-thiophene) (rrP3HT) and multiwall carbon nanotubes have been investigated by scanning tunneling microscopy in ultrahigh vacuum. Carbon nanotubes covered by rrP3HT have been imaged and analyzed, providing a clear evidence that this polymer self-assembles on the nanotube surface following geometrical constraints and adapting its equilibrium chain-to-chain distance. Largely spaced covered nanotubes have been analyzed to investigate the role played by nanotubechirality in the polymer wrapping, evidencing strong rrP3HT interactions along well defined directions.
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