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cluster formation at interfaces with pentacene thin-film phases
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/content/aip/journal/apl/95/21/10.1063/1.3266857
2009-11-24
2014-09-03

Abstract

The -thin film pentacene interface was investigated using scanning tunneling microscopy,atomic force microscopy, and ultraviolet photoemission spectroscopy. deposition on a multilayer pentacene film (standing) yields an interface dominated by clusters, regardless of the underlying substrate. Three-dimensional cluster growth dominates due to weak interactions with the underlying Pn. cluster size and density on sequential Pn layers suggest an Ehrlich–Schwoebel-type barrier at Pn layer boundaries. Cluster formation reduces the lowest unoccupied molecular orbital–Pn highest occupied molecular orbital (HOMO) separation, while increasing the respective HOMO-HOMO offset. Heterostructure fabrication protocols can alter interface morphology and induce band shifts on the order of 0.3 eV.

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Scitation: C60 cluster formation at interfaces with pentacene thin-film phases
http://aip.metastore.ingenta.com/content/aip/journal/apl/95/21/10.1063/1.3266857
10.1063/1.3266857
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