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Single-beam coherent anti-Stokes Raman scattering spectroscopy of using a shaped 7 fs laser pulse
1.A. C. Eckbreth, Laser Diagnostics for Combustion Temperature and Species, 2nd ed. (Gordon and Breach, Amsterdam, 1996).
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The feasibility is explored by single-beam coherent anti-Stokes Raman scattering (CARS)spectroscopy of gas-phase diatomic molecules related to combusting flows, with implications for gas-phase thermometry. We demonstrate CARS of gas-phase using a shaped laser pulse, investigate the dependence of the CARS signal on the total pressure of the probed environment, both in pure and in mixtures with Ar, discuss the observed signal-to-noise ratio, and suggest improvements to be considered for reliable single-shot measurements at flame temperatures.
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