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Multiply-resonant nonlinear optical processes in doped polythiophenes
3.T. Yamamoto, Z. Zhou, T. Kanbara, M. Shimura, K. Kizu, T. Maruyama, Y. Nakamura, T. Fukuda, B. L. Lee, N. Ooba, S. Tomaru, T. Kurihara, T. Kaino, K. Kubota, and S. Sasaki, J. Am. Chem. Soc. 118, 10389 (1996).
23.P. N. Butcher and D. Cotter, The Elements of Nonlinear Optics (Cambridge University Press, Cambridge, 1990).
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We investigated the third-order optical nonlinearity in chemically doped poly(3-hexylthiophenes) by the third-harmonic generation (THG) method. The THG spectra reveal that the third-order optical nonlinearity is governed by the polaron states. The spectral analysis clarified the occurrence of multiple resonance related to transitions to the polaron states and the transition.
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