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/content/aip/journal/aplmater/3/10/10.1063/1.4931487
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/content/aip/journal/aplmater/3/10/10.1063/1.4931487
2015-09-18
2016-09-30

Abstract

A series of cation-doped BaTaON particle was synthesized to control the donor density in the bulk for improving the performance of photoelectrochemical water splitting on porous BaTaON photoanodes under visible light. Among the dopants (Mo 6+, W6+, Zr4+, and Ti4+) examined, Mo 6+ cations can be introduced into the Ta 5+ site up to 5 mol. % without producing any impurity phases; the donor density of BaTaON was indeed increased significantly by introducing higher ratio of Mo 6+ dopant. The porous photoanodes of Mo-doped BaTaON showed much higher photocurrent than others including undoped one and also exhibited much improved performance in photoelectrochemical water splitting into H and O after loaded with cobalt oxide cocatalyst and coupled with Pt counter electrode.

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