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/content/aip/journal/aplmater/3/4/10.1063/1.4913395
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/content/aip/journal/aplmater/3/4/10.1063/1.4913395
2015-02-24
2016-09-27

Abstract

New 3 transition metal-based mixed-pnictide compounds, La AsN ( = Fe, Co, and Ni) are synthesized by solid state reactions under a high pressure of 2.5 GPa. These compounds crystallize with an orthorhombic structure (space group mcm) containing four formula units per unit cell. The crystal structure consists of an anisotropic network of AsN tetrahedra sharing As-As edges along the in-plane direction and N corners along the -direction, forming a honeycomb lattice with a boat-shape conformation bridged by -N- linear bonds. The temperature dependences of the electrical resistivity and magnetic susceptibility indicate that these crystals are itinerant antiferromagnets exhibiting parasitic ferromagnetism with transition temperatures of 560, 260, and 410 K for = Fe, Co, and Ni, respectively. These compounds are expected to be parent materials for new superconductors.

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