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BiTe-based compounds are a well-known class of outstanding thermoelectric materials. β-AsTe, another member of this family, exhibits promising thermoelectric properties around 400 K when appropriately doped. Herein, we investigate the high-temperature thermoelectric properties of the β-AsBiTe solid solution. Powder X-ray diffraction and scanning electron microscopy experiments showed that a solid solution only exists up to = 0.035. We found that substituting Bi for As has a beneficial influence on the thermopower, which, combined with extremely low thermal conductivity values, results in a maximum value of 0.7 at 423 K for = 0.017 perpendicular to the pressing direction.


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