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Quantum dots embedded into silicon nanowires effectively partition electron confinement
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10.1063/1.2973464
/content/aip/journal/jap/104/5/10.1063/1.2973464
http://aip.metastore.ingenta.com/content/aip/journal/jap/104/5/10.1063/1.2973464

Figures

Image of FIG. 1.
FIG. 1.

(a) Atomic structure of silicon nanowires, illustrated for and . describes the number of prism layers in the nanowire cross section (1 and 2). gives the number of the lengthwise segments (1, 2, 3, and 4). The asterisk denotes the formation of silicon dimers on the facets of the nanowires. (b) Quantum dot with the 20-atom core of symmetry (shown in red sticks). is the number of layers of silicon atoms including the core. (c) Side and top views of the quantum dot attached to the nanowire . The silicon atoms of the quantum dot, nanowire and the shared interface are shown in red (gray off line), blue (black off line), and green (light gray off line), respectively. Hydrogen atoms are not shown.

Image of FIG. 2.
FIG. 2.

(a) Scanning electron microscopy image of a branched silicon nanowire (adapted from Ref. 10 and reproduced pending the permission from Nano Lett.). b) Atomic structures of silicon nanowires with embedded quantum dots (see main text for the notation). The linear sizes of the schematic systems are shown for some actual systems, along with their diameters . Only very few of the computed systems are illustrated, and the sizes and symmetry of all systems are provided in Table I. Silicon and hydrogen atoms are shown in red and blue, respectively.

Image of FIG. 3.
FIG. 3.

Band gap energy dependence on the linear size , showing the quantum confinement effect in (a) simple nanowires : black lines with circles, : red lines with triangles, and complex connected nanowires : green lines with squares; (b) quantum dot–nanowire junctions of : green lines with triangles, : black lines with circles, : red lines with circles, and : red lines with triangles and blue lines with squares . Numbers show the number of segments in nanowires. Pairs of numbers are given if more than one nanowire is present, giving the two independent numbers of segments. pairs are equivalent to single and are so shown to elucidate the structure connection.

Image of FIG. 4.
FIG. 4.

(a) Total and partial DOS of complex nanoclusters. Partial DOS are shown in the same color as the corresponding atomic structures. (b) The detailed total and partial DOS of occupied electronic states of cluster near the Fermi level region. Peaks , , and correspond to the , , and fragments respectively.

Image of FIG. 5.
FIG. 5.

Molecular orbital diagram elucidating the quantum confinement. When system is elongated with producing , nearly degenerate occupied and virtual orbitals are shifted by the interaction (e.g., the HOMO and LUMO orbital energies shifted by and , respectively), reducing the band gap from to .

Tables

Generic image for table
Table I.

Atomic and electronic structure of complex nanostructures.

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/content/aip/journal/jap/104/5/10.1063/1.2973464
2008-09-08
2014-04-19
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Quantum dots embedded into silicon nanowires effectively partition electron confinement
http://aip.metastore.ingenta.com/content/aip/journal/jap/104/5/10.1063/1.2973464
10.1063/1.2973464
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