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Time-dependent investigation of charge injection in a quantum dot containing one electron
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10.1063/1.4759292
/content/aip/journal/jap/112/9/10.1063/1.4759292
http://aip.metastore.ingenta.com/content/aip/journal/jap/112/9/10.1063/1.4759292

Figures

Image of FIG. 1.
FIG. 1.

Schematics of an injected electron state in the form of a gaussian wave packet (half-width of ) with a kinetic energy moving towards a QD (of width W) containing one electron in one of the confined states. The depth of the confining potential is (represented by the solid red line). The effective potential for the injected electron is represented by the dashed red line. The green arrows represent the possible quantum transitions that the confined electron may undergo due to the interaction with the injected electron. There are two types of transitions: (i) intersubband transitions for the case that the electron is excited from the ground to the first excited QD state, and (ii) ionization, for the case where the confined electron is excited to a delocalized continuum state. The whole system is embedded in a quantum wire of diameter D (see upper inset). In this work, we have adopted , and . The barrier sizes are of the order of 30 nm, and the size of the absorbing layers is 5 nm which are introduced in order to eliminate spurious reflections.

Image of FIG. 2.
FIG. 2.

Effective Coulomb potential for and different values of the dielectric constant of the semiconductor, and different diameters D of the quantum dot.

Image of FIG. 3.
FIG. 3.

Matrix form of the system of time dependent equations given by Eq. (3) where .

Image of FIG. 4.
FIG. 4.

(left)Time evolution of for different energies of the injected electron (0.1 eV and 0.5 eV) at intervals of 8 fs. The initial state has a single component (), such that no transitions between the angular modes are allowed. The QD dimensions are W = 3 nm, D = 10 nm, and the dielectric constant is . The width of the injected particle is . (right-top) Position-dependent probability to find either particle in the z direction within the time window up to 40 fs. The vertical dashed lines represent the QD region. The horizontal dotted lines are reference lines. (right-bottom) Momentum-dependent probability to find either particle with a momentum k.

Image of FIG. 5.
FIG. 5.

(top) Time dependence of the average position of the particle confined in the QD for different kinetic energies of the injected particle. (middle) Average position of the position-dependent probability . (bottom) Average momentum of the incident (solid curves) and transmitted (dashed curves) total wave function for different kinetic energies of the injected particle. The QD parameters are the same as for Fig. 4.

Image of FIG. 6.
FIG. 6.

Region-dependent probability to find one electron in the left (), center () and right () sides with respect to the QD position. The sum of these probabilities is also shown (solid circles). The parameters are the same as for Fig. 4. The injected kinetic energies are: 0.1 eV (black), 0.5 eV (blue), and 1.0 eV (red). The vertical lines mark the maximum traveling time of the total wave function before is drained by the absorbing layers. is also used to determine the transmission and reflection coefficients as and , respectively. represents the peak of .

Image of FIG. 7.
FIG. 7.

(top) Dependence of P (solid), T (dashed), and R (dash-dotted) coefficients on the kinetic energy of the injected particle. Results are shown for different QD widths: W = 3 nm (black), W = 5 nm (blue), and W = 7 nm (red). The QD diameters are D = 5 nm (so symbol) and D = 10 nm (circle). (bottom) Energy dependence of the peak probability of (see Fig. 6). The diameter dependence is negligible for . Here we used .

Image of FIG. 8.
FIG. 8.

Difference of P (solid), T (dashed) and R (dash-dotted) calculated with and without the Coulomb interaction for D = 10 nm. Different QD widths are shown: W = 3 nm (black), W = 5 nm (blue), and W = 7 nm (red). Here we used .

Image of FIG. 9.
FIG. 9.

Dependence of P (solid), T (dashed), and R (dash-dotted) on the half-width of the incident wave packet for kinetic energy . Different QD widths are shown: W = 3 nm (black), W = 5 nm (blue), and W = 7 nm (red). The QD diameter is D = 10 nm. Here we used .

Image of FIG. 10.
FIG. 10.

Dependence of P (solid), T (dashed), and R (dash-dotted) on the dielectric constant for a kinetic energy of . Different values of are shown: (black), (blue), and (red). The QD dimensions are D = 10 nm and W = 3 nm.

Image of FIG. 11.
FIG. 11.

Characteristic transition time of a Coulomb mediated intersubband transition between the two lowest confined states in the QD. The QD dimensions are W = 3 nm and D = 10 nm.

Tables

Generic image for table
Table I.

Indexing scheme of the lowest two-electron radial states (i,j) in terms of the single-particle radial quantum numbers.

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/content/aip/journal/jap/112/9/10.1063/1.4759292
2012-11-02
2014-04-23
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Time-dependent investigation of charge injection in a quantum dot containing one electron
http://aip.metastore.ingenta.com/content/aip/journal/jap/112/9/10.1063/1.4759292
10.1063/1.4759292
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