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Local structure around rare-earth ions in B2O3 glass at high pressure
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10.1063/1.4811185
/content/aip/journal/jap/113/22/10.1063/1.4811185
http://aip.metastore.ingenta.com/content/aip/journal/jap/113/22/10.1063/1.4811185
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Optical microscope images of BO glass with 0.1 mol. % YbO prepared at 0.1 MPa.

Image of FIG. 2.
FIG. 2.

Natural logarithm of reciprocal of optical transmittance of BO glasses with 0.1 mol. % REO of 2 mm in thickness prepared at 0.1 MPa (a) and 3 GPa (b), and calculated scattering spectra of BO glasses including REO·3BO particles of various diameters; 0.1, 0.2, 0.5, 1, 2, and 5 m(c).

Image of FIG. 3.
FIG. 3.

Photoluminescence spectra of RE ions in BO glasses prepared at 0.1 MPa and 3 GPa; RE = Ce (a), Sm (b), Eu (c), Eu (d), and Dy(e).

Image of FIG. 4.
FIG. 4.

Optical absorption spectra of BO glass with 0.1 mol. % DyO prepared at 3 GPa (a) and 0.1DyO·NaO·(100 − )BO glasses of  = 10 (b), 20 (c), and 30 (d) prepared at 0.1 MPa, and Judd-Ofelt parameters of the above glasses (e).

Image of FIG. 5.
FIG. 5.

Measured ESE spectra (a), ESEEM spectra (b), and Fourier transform spectra (c) of BO glasses with 0.1 mol. % CeO prepared at 0.1 MPa and 3 GPa and 0.1DyO·NaO·(100 − )BO glasses of  = 10, 20, and 30 prepared at 0.1 MPa. The arrows indicate the Larmor frequencies at 500 mT of the nuclear atoms; B, B, and Na.

Image of FIG. 6.
FIG. 6.

Calculated ESEEM spectra of ligands; BO, BO, BOO, and Na (a), experimental (○) and simulated (―) ESEEM spectra of BO glasses with 0.1 mol. % CeO prepared at 0.1 MPa (b) and 3 GPa (c) and 0.1DyO·NaO·(100 − )BO glasses of  = 10 (d), 20 (e), and 30 (f) prepared at 0.1 MPa, and estimated numbers of BO, BO, BOO, and Na around a cerium ion in the above glasses (g).

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/content/aip/journal/jap/113/22/10.1063/1.4811185
2013-06-13
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Local structure around rare-earth ions in B2O3 glass at high pressure
http://aip.metastore.ingenta.com/content/aip/journal/jap/113/22/10.1063/1.4811185
10.1063/1.4811185
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