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Dynamic arrest in a liquid of symmetric dumbbells: Reorientational hopping for small molecular elongations
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10.1063/1.2085030
/content/aip/journal/jcp/123/20/10.1063/1.2085030
http://aip.metastore.ingenta.com/content/aip/journal/jcp/123/20/10.1063/1.2085030
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Top panel: Isodiffusivity lines (thin continuous lines) and (thin dotted lines) and (thick dotted lines) isochrones in the plane. These quantities are averaged over all the particles in the system. Line segments join the numerical data (symbols are not included for clarity). The corresponding values are, from top to bottom, , , , , and , , , , , , , , and , and , , , , , and . The empty and filled symbols are, respectively, the estimated MCT and VFT temperatures (see text) for (circles), (squares), and (triangles). The thick dashed and thick continuous lines are corresponding guides for the eyes. The lower panel shows a magnification, for , of the results in the neighborhood of the estimated MCT transition temperatures.

Image of FIG. 2.
FIG. 2.

Symbols: Temperature dependence of (a), (b), and (c). The continuous lines are fits to the VFT functions (see text). The dashed lines in panel (b) are Arrhenius fits. The data for have been represented vs in order to show the Arrhenius behavior at small .

Image of FIG. 3.
FIG. 3.

Temperature dependence of the rotational correlators and vs time rescaled by , for elongation . From top to bottom , 0.276, 0.343, 0.496, 0.750, 1.110, 1.396, 1.693, 1.770, 1.815, 1.933, 2.443, and 3.776.

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/content/aip/journal/jcp/123/20/10.1063/1.2085030
2005-11-28
2014-04-23
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Dynamic arrest in a liquid of symmetric dumbbells: Reorientational hopping for small molecular elongations
http://aip.metastore.ingenta.com/content/aip/journal/jcp/123/20/10.1063/1.2085030
10.1063/1.2085030
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