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Photoelectron spectroscopy of toluene: II. Intramolecular dynamics of selected vibrational levels in toluene studied by nanosecond and picosecond time-resolved photoelectron spectroscopies
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10.1063/1.2126974
/content/aip/journal/jcp/123/20/10.1063/1.2126974
http://aip.metastore.ingenta.com/content/aip/journal/jcp/123/20/10.1063/1.2126974
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Photoelectron spectra (from time of flight) following the excitation of the upper component of the Fermi coupled pair at and ionization with the same wavelength. Upper panel: excitation and ionization with overlapped duration laser pulses; lower panel: excitation and ionization with overlapped duration laser pulses.

Image of FIG. 2.
FIG. 2.

Photoelectron spectra (from time of flight) following the excitation of the (left) and (right) levels at 935 and , respectively, and ionization with the excitation wavelength. Upper panel: excitation and ionization with overlapped duration laser pulses; lower panel: excitation and ionization with overlapped duration laser pulses.

Image of FIG. 3.
FIG. 3.

Picosecond time-resolved photoelectron spectra (from time of flight) following the excitation of (left) the level in toluene at and (right) the level in toluene at . “X” denotes either or in the ion, or both together, as they cannot be distinguished.

Image of FIG. 4.
FIG. 4.

Photoelectron spectra (from time of flight) following the excitation of the level at and ionization at the same wavelength. Upper panel: excitation and ionization with overlapped duration laser pulses; lower panel: excitation and ionization with overlapped duration laser pulses.

Image of FIG. 5.
FIG. 5.

Picosecond time-resolved photoelectron spectra (from time of flight) following the excitation of (left) the level in toluene at and (right) the level in -fluorotoluene at .

Image of FIG. 6.
FIG. 6.

Velocity-map image photoelectron spectra following the preparation and ionization of the toluene origin with overlapped laser pulses at the same wavelength. Top: seeded molecular beam; bottom: effusive source.

Image of FIG. 7.
FIG. 7.

Time-of-flight photoelectron spectra following the preparation and ionization of the toluene origin with overlapped laser pulses at the same wavelength. Top: seeded molecular beam; bottom: ambient sample.

Image of FIG. 8.
FIG. 8.

Nanosecond time-resolved velocity-map image photoelectron spectra following the preparation of the toluene origin and ionization at . The dotted line in the upper three traces indicates the spectrum.

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/content/aip/journal/jcp/123/20/10.1063/1.2126974
2005-11-29
2014-04-17
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Photoelectron spectroscopy of S1 toluene: II. Intramolecular dynamics of selected vibrational levels in S1 toluene studied by nanosecond and picosecond time-resolved photoelectron spectroscopies
http://aip.metastore.ingenta.com/content/aip/journal/jcp/123/20/10.1063/1.2126974
10.1063/1.2126974
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