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Temperature- and species-dependent quenching of NO probed by two-photon laser-induced fluorescence using a picosecond laser
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10.1063/1.2206783
/content/aip/journal/jcp/124/23/10.1063/1.2206783
http://aip.metastore.ingenta.com/content/aip/journal/jcp/124/23/10.1063/1.2206783

Figures

Image of FIG. 1.
FIG. 1.

Experimental arrangement for time-resolved picosecond LIF detection of NO. Gr, grating; Pr, prism; BPF, bandpass filter; Ap, aperture.

Image of FIG. 2.
FIG. 2.

Two measurements of the quenching rate coefficient for at . The upper pressure sequence is offset vertically by for clarity.

Image of FIG. 3.
FIG. 3.

Calculated and measured fluorescence decay rates in a methane/air counterflow diffusion flame (Ref. 15). The error bar represents the typical measurement uncertainty in the flame zone.

Image of FIG. 4.
FIG. 4.

Temperature dependence of the self-quenching cross section. The fitting function and parameters listed in Table VIII produced the solid curve. Inset displays data and models for up to .

Image of FIG. 5.
FIG. 5.

Temperature dependence of quenching cross section. The fitting function and parameters listed in Table VIII produced the solid curve.

Image of FIG. 6.
FIG. 6.

Temperature dependence of quenching cross section. The fitting function and parameters listed in Table VIII produced the solid curve.

Image of FIG. 7.
FIG. 7.

Temperature dependence of quenching cross section. The fitting function and parameters listed in Table VIII produced the solid curve.

Image of FIG. 8.
FIG. 8.

Temperature dependence of CO quenching cross section. The fitting function and parameters listed in Table VIII produced the solid curve.

Image of FIG. 9.
FIG. 9.

Temperature dependence of quenching cross section. The fitting function and parameters listed in Table VIII produced the solid curve. Inset displays data and models for up to .

Image of FIG. 10.
FIG. 10.

Temperature dependence of quenching cross section. The fitting function and parameters listed in Table VIII produced the solid curve.

Tables

Generic image for table
Table I.

Summary of self-quenching measurements. Values listed in parentheses represent fitting uncertainty.

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Table II.

Summary of quenching from 245 decay-rate measurements. Values listed in parentheses represent fitting uncertainty.

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Table III.

Summary of quenching from 311 decay-rate measurements. Values listed in parentheses represent fitting uncertainty.

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Table IV.

Summary of quenching from 188 decay-rate measurements. Values listed in parentheses represent fitting uncertainty.

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Table V.

Summary of CO quenching from 209 decay-rate measurements. Values listed in parentheses represent fitting uncertainty.

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Table VI.

Summary of quenching from 153 decay-rate measurements. Values listed in parentheses represent fitting uncertainty.

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Table VII.

Summary of quenching from 118 decay-rate measurements. Values listed in parentheses represent fitting uncertainty.

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Table VIII.

Empirical models for the temperature dependence of quenching cross sections.

Generic image for table
Table IX.

Prior experimental determinations of NO lifetime.

Generic image for table
Table X.

Legend for Figs. 4–10.

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/content/aip/journal/jcp/124/23/10.1063/1.2206783
2006-06-19
2014-04-16
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Temperature- and species-dependent quenching of NO AΣ+2(v′=0) probed by two-photon laser-induced fluorescence using a picosecond laser
http://aip.metastore.ingenta.com/content/aip/journal/jcp/124/23/10.1063/1.2206783
10.1063/1.2206783
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