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Photodissociation dynamics of pyrimidine
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10.1063/1.2174011
/content/aip/journal/jcp/124/8/10.1063/1.2174011
http://aip.metastore.ingenta.com/content/aip/journal/jcp/124/8/10.1063/1.2174011

Figures

Image of FIG. 1.
FIG. 1.

Photofragment ion images from the photodissociation of pyrimidine at . The wavelength of the vuv laser is .

Image of FIG. 2.
FIG. 2.

Photofragment ion images from the photodissociation of pyrimidine at . The wavelength of the vuv laser is .

Image of FIG. 3.
FIG. 3.

Total translational energy distributions of reactions obtained at . (a) . Only was measured. (b) . (c) . (d) . (e) . (f) . Except (a) which only was measured, both fragments were measured for the other channels.

Image of FIG. 4.
FIG. 4.

Intensity changes of these disklike images as well as the product growth with respect to the delay time between pump and probe laser pulses. The photolysis wavelength is ; the wavelength of the vuv laser is . The solid squares are the experimental data. The solid lines are the fit to .

Image of FIG. 5.
FIG. 5.

Photofragment ion images from the photodissociation of pyrimidine at . The wavelength of the vuv laser is .

Image of FIG. 6.
FIG. 6.

Total translational energy distributions of reactions obtained at . (a) . (b) . (c) . (d) . Translational energy smaller than is obscured by the disklike image. For (a) and (b), only heavy fragments were measured. Only light fragment in (d) was measured.

Image of FIG. 7.
FIG. 7.

Intensity changes of these disklike images as well as the product growth with respect to the delay time between pump and probe laser pulses. The photolysis wavelength is ; the wavelength of the vuv laser is . The solid squares are the experimental data. The solid lines are the fit to .

Image of FIG. 8.
FIG. 8.

Potential energies (in kcal/mol) and structures of products for H atom elimination.

Image of FIG. 9.
FIG. 9.

Potential energies (in kcal/mol) and structures of intermediates and products for and HCN.

Image of FIG. 10.
FIG. 10.

Potential energies (in kcal/mol) and structures of intermediates and products for .

Image of FIG. 11.
FIG. 11.

Potential energies (in kcal/mol) and structures of intermediates and products for .

Image of FIG. 12.
FIG. 12.

Potential energies (in kcal/mol) and structures of intermediates and products for .

Image of FIG. 13.
FIG. 13.

Potential energies (in kcal/mol) and structures of intermediates and products for .

Tables

Generic image for table
Table I.

Ion intensity ratios from .

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/content/aip/journal/jcp/124/8/10.1063/1.2174011
2006-02-22
2014-04-16
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Photodissociation dynamics of pyrimidine
http://aip.metastore.ingenta.com/content/aip/journal/jcp/124/8/10.1063/1.2174011
10.1063/1.2174011
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