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Fundamental limits of all nonlinear-optical phenomena that are representable by a second-order nonlinear susceptibility
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10.1063/1.2358973
/content/aip/journal/jcp/125/15/10.1063/1.2358973
http://aip.metastore.ingenta.com/content/aip/journal/jcp/125/15/10.1063/1.2358973
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

(Color) The dispersion of (a) the real part and (b) the imaginary part of fundamental limit of the hyperpolarizability normalized to the off-resonant limit with , , and for a one-electron system.

Image of FIG. 2.
FIG. 2.

(Color) The real part of fundamental limit of the electro-optic hyperpolarizability normalized to the off-resonant limit with as a function of for various values of .

Image of FIG. 3.
FIG. 3.

(Color) The real part of the fundamental limit of the second harmonic hyperpolarizability normalized to the off-resonant limit with as a function of for various off-resonant pump wavelengths.

Image of FIG. 4.
FIG. 4.

Off-resonant as a function of and the energy of the second excited state with homogeneous width [given by Eq. (19)] and .

Image of FIG. 5.
FIG. 5.

The second harmonic hyperpolarizability as a function of and the energy to the second excited state . The inset in the bottom plot shows the energy level diagram and excitation photons, with the shaded region representing the calculated range of the second excited state energy.

Image of FIG. 6.
FIG. 6.

(Color) The second harmonic hyperpolarizability as a function of and the energy to the second excited state with .

Image of FIG. 7.
FIG. 7.

The fundamental limit of the second harmonic hyperpolarizability as a function of and the second excited state energy when the first excited state is at . The inset shows the virtual excitation diagram of the process, where the gray region depicts the range of .

Image of FIG. 8.
FIG. 8.

The fundamental limit of the second harmonic hyperpolarizability as a function of and the second excited state energy when the first excited state is at . The inset shows the virtual excitation diagram of the process, where the gray region depicts the range of .

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/content/aip/journal/jcp/125/15/10.1063/1.2358973
2006-10-19
2014-04-20
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Fundamental limits of all nonlinear-optical phenomena that are representable by a second-order nonlinear susceptibility
http://aip.metastore.ingenta.com/content/aip/journal/jcp/125/15/10.1063/1.2358973
10.1063/1.2358973
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