Mode-dependent enhancement of photodissociation and photoionization in a seven atom molecule
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Vibrational excitation of the stretch region of methylamine: (a) room temperature photoacoustic Raman spectrum, (b) jet-cooled action spectrum monitoring the yield of H photofragments following photodissociation of pre-excited methylamine and (c) resonantly enhanced multi-photon ionization spectrum. The insets display simple diagrams of the excitation scheme used to obtain each spectrum, where the potential energy surfaces for dissociation are adopted from Ref. 17, the dashed line denoting symmetry and the solid line symmetry.
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