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Probing the valence character of O excited by participator Auger decay measurements and partial ion yield spectroscopy following x-ray absorption
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10.1063/1.2723745
/content/aip/journal/jcp/126/17/10.1063/1.2723745
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/17/10.1063/1.2723745
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Figures

Image of FIG. 1.
FIG. 1.

A high-resolution oxygen -edge total ion yield photoabsorption spectrum of recorded in the photon energy range between 537 and . The selected photon energies for the recording of resonant Auger participator decay spectra are numbered for orientation.

Image of FIG. 2.
FIG. 2.

Normalized resonant Auger electron spectra (cf. Sec. II) showing the valence spectral region between 10 and binding energy, recorded on top of peaks 1–5 of Fig. 1 (, 540.24, 540.66, 540.88, and , respectively). An off-resonance spectrum recorded at photon energy is also included for comparison.

Image of FIG. 3.
FIG. 3.

A blowup of the state recorded at resonance peak 1 . Teeth of the comb represent calculated vibrational energies based on the spectroscopic constants derived in this work (see text).

Image of FIG. 4.
FIG. 4.

Normalized resonant Auger electron spectra (cf. Sec. II) showing the valence spectral region between 10 and binding energy, recorded on top of peaks 6–10 of Fig. 1 (, 541.97, 542.26, 542.50, and , respectively). An off-resonance spectrum recorded at photon energy is also included for comparison.

Image of FIG. 5.
FIG. 5.

(Color online) High-resolution, oxygen -edge and ion yield photoabsorption spectra of recorded in the photon energy range between 537 and . Also included are the values of the integrated areas of the state (, filled circles), the three overlapping , , and states (, empty triangles), the state (, filled triangles), and the state (, empty circles) as extracted from Figs. 2 and 4, respectively.

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/content/aip/journal/jcp/126/17/10.1063/1.2723745
2007-05-02
2014-04-20
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Probing the valence character of O 1s→Rydberg excited O2 by participator Auger decay measurements and partial ion yield spectroscopy following x-ray absorption
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/17/10.1063/1.2723745
10.1063/1.2723745
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