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Analysis of cross peaks in two-dimensional electronic photon-echo spectroscopy for simple models with vibrations and dissipation
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10.1063/1.2435353
/content/aip/journal/jcp/126/7/10.1063/1.2435353
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/7/10.1063/1.2435353
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Ground-state and excited-state potential-energy surfaces for the system mode. Several vibrational levels are indicated for each electronic state.

Image of FIG. 2.
FIG. 2.

2D electronic photon-echo spectra of (a) the two-state model (weakly damped displaced harmonic oscillator) and (b) the three-state model, calculated in the quasi-impulsive limit for zero temperature and weak optical dephasing . Correlation spectra as well as relaxation spectra for , 200, and are shown. The transition dipole moments are in (a) and and in (b). The frequency scale is in eV and corresponds to transition frequencies reduced by .

Image of FIG. 3.
FIG. 3.

2D electronic photon-echo correlation spectra of [(a) and (b)] the two-state model (weakly damped displaced harmonic oscillator) and [(c)–] the three-state model, calculated with pulse durations [short pulses, (a)–(d)] and [long pulses, (a)–], for zero temperature and weak optical dephasing . The reduced carrier frequencies of the pulses are in (a) and in (b)–. The transition dipole moments are in [(a) and (b)], and in (c), and in (d), and and in . The frequency scale is in eV and corresponds to transition frequencies reduced by .

Image of FIG. 4.
FIG. 4.

2D electronic photon-echo correlation spectra of (a) the two-state model (weakly damped displaced harmonic oscillator) and [(b) and (c)] the three-state model, calculated with pulse durations (quasi-impulsive limit), (short pulses), and (long pulses), for zero temperature and strong optical dephasing . The reduced carrier frequencies of the pulses are . The transition dipole moments are in (a), in (b) and (c), in (b), and in (c). The frequency scale is in eV and corresponds to transition frequencies reduced by .

Image of FIG. 5.
FIG. 5.

2D electronic photon-echo correlation spectra of the three-state model, calculated with pulse durations (a) (quasi-impulsive limit), (b) (short pulses), and (c) (long pulses), temperatures of 300 and , and weak optical dephasing . The reduced carrier frequencies of the pulses are . The transition dipole moments are and in (a), and in (b), and and in (c). The frequency scale is in eV and corresponds to transition frequencies reduced by .

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/content/aip/journal/jcp/126/7/10.1063/1.2435353
2007-02-21
2014-04-20
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Analysis of cross peaks in two-dimensional electronic photon-echo spectroscopy for simple models with vibrations and dissipation
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/7/10.1063/1.2435353
10.1063/1.2435353
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