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Fragmentation dynamics of methane by few-cycle femtosecond laser pulses
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10.1063/1.2472341
/content/aip/journal/jcp/126/7/10.1063/1.2472341
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/7/10.1063/1.2472341
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

(a) Spectrum and (b) interferometric autocorrelation (IAC) of the ultrashort laser pulse. The spectrum was not calibrated with the response curve of the detector.

Image of FIG. 2.
FIG. 2.

Time-of-flight mass spectra of methane irradiated by different pulse durations and comparable peak laser intensities. (a) and , (b) and , and (c) and . The spectra were normalized to the intensity of the . Please note that the signal of was divided by 4 for laser pulses.

Image of FIG. 3.
FIG. 3.

Potential energy surfaces of at different laser intensities and in two opposite laser field directions. The field vector is shown by the arrows: (a) and (b) .

Image of FIG. 4.
FIG. 4.

Time-dependent dissociation probability for the C–H bond parallel to the laser polarization direction at different laser intensities.

Image of FIG. 5.
FIG. 5.

Field-free potential energy surfaces of .

Image of FIG. 6.
FIG. 6.

Time-of-flight mass spectra of irradiated by laser pulse at (a) , (b) , and (c) . The spectra were normalized to the intensity of . The intensities were magnified by 20 for the mass peaks of , , and .

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/content/aip/journal/jcp/126/7/10.1063/1.2472341
2007-02-21
2014-04-19
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Fragmentation dynamics of methane by few-cycle femtosecond laser pulses
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/7/10.1063/1.2472341
10.1063/1.2472341
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