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Energy dependent decay rates of Lennard-Jones clusters for use in nucleation theory
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10.1063/1.2698424
/content/aip/journal/jcp/126/7/10.1063/1.2698424
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/7/10.1063/1.2698424
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Natural logarithm of fraction of decamers surviving vs dimensionless time for various dimensionless collision frequencies of thermalizing gas molecules. The dotted line is the average decay rate , and the triangles show values from Eq. (5).

Image of FIG. 2.
FIG. 2.

Natural logarithm of fraction of decamers of given energy surviving vs dimensionless time for various total cluster energies (in units of ), .

Image of FIG. 3.
FIG. 3.

Energy dependent decay rates vs total cluster energy for (triangles), 20 (circles), 30 (squares), and 40 (diamonds) from molecular dynamics simulations. The dotted lines show the values calculated from Eq. (9).

Image of FIG. 4.
FIG. 4.

Normalized energy distributions of clusters at temperature . The solid lines are values from the Monte Carlo method and the dotted lines are Gaussian fits [Eq. (8)], using the mean and standard deviation of the Monte Carlo runs.

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/content/aip/journal/jcp/126/7/10.1063/1.2698424
2007-02-21
2014-04-20
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Energy dependent decay rates of Lennard-Jones clusters for use in nucleation theory
http://aip.metastore.ingenta.com/content/aip/journal/jcp/126/7/10.1063/1.2698424
10.1063/1.2698424
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