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Development of the energy flow in light-harvesting dendrimers
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10.1063/1.2785175
/content/aip/journal/jcp/127/13/10.1063/1.2785175
http://aip.metastore.ingenta.com/content/aip/journal/jcp/127/13/10.1063/1.2785175
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

First-generation dendrimers, , , and .

Image of FIG. 2.
FIG. 2.

Extent of core excitation as a function of the iteration count, for different values of propensities , , and in the matrix (1).

Image of FIG. 3.
FIG. 3.

Core excited state population scaled by the total number of chromophores in dendrimers of vertex degree , plotted as a function of the directional efficiency of intershell RET, for three-, four-, and five-generation dendrimers.

Image of FIG. 4.
FIG. 4.

Core excitation of a three-generation dendrimer [described by Eqs. (16) and (17)], plotted as a function of (measure of the spectroscopic gradient) for different values of (the relative Stokes shift).

Image of FIG. 5.
FIG. 5.

Time evolution of the excited core population, for and 0.8, for (i) two-generation, (iii) three-generation, and (v) four-generation dendrimers, and their respective increases in core excitation per unit time (ii), (iv), and (vi). The parameter values are , for , , and .

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/content/aip/journal/jcp/127/13/10.1063/1.2785175
2007-10-03
2014-04-25
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Development of the energy flow in light-harvesting dendrimers
http://aip.metastore.ingenta.com/content/aip/journal/jcp/127/13/10.1063/1.2785175
10.1063/1.2785175
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