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Elucidating the spectral and temporal contributions from the resonant and nonresonant response to femtosecond coherent anti-Stokes Raman scattering
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10.1063/1.2897975
/content/aip/journal/jcp/128/15/10.1063/1.2897975
http://aip.metastore.ingenta.com/content/aip/journal/jcp/128/15/10.1063/1.2897975
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Figures

Image of FIG. 1.
FIG. 1.

The spectra measured for for selected detunings. (a) and (b) . The spectra are shifted for clarity. The vertical dashed line corresponds to the resonant CARS photon energy expected from the transition. Insets show corresponding energy level diagram for the CARS process.

Image of FIG. 2.
FIG. 2.

The spectra predicted using Eq. (3) for the detunings presented in Fig. 1. (a) and (b) . The spectra are shifted for clarity.

Image of FIG. 3.
FIG. 3.

(a) spectra at different negative delays . (b) spectra at different positive delays . Insets show the corresponding sequence of the arrival of two pump beams and Stokes beam. All spectra are taken at (nearly below the resonance).

Image of FIG. 4.
FIG. 4.

CARS spectra of the oxygen vibrational transition . Circles are experimental points for with the dashed line representing the theoretical fit from Eq. (3). Squares are experimental points for and the solid line is the theoretical fit from Eq. (3) with .

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/content/aip/journal/jcp/128/15/10.1063/1.2897975
2008-04-18
2014-04-19
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Elucidating the spectral and temporal contributions from the resonant and nonresonant response to femtosecond coherent anti-Stokes Raman scattering
http://aip.metastore.ingenta.com/content/aip/journal/jcp/128/15/10.1063/1.2897975
10.1063/1.2897975
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