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Perturbative theory and modeling of electronic-resonance-enhanced coherent anti-Stokes Raman scattering spectroscopy of nitric oxide
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10.1063/1.2909554
/content/aip/journal/jcp/128/17/10.1063/1.2909554
http://aip.metastore.ingenta.com/content/aip/journal/jcp/128/17/10.1063/1.2909554
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

CARS energy-level diagram including electronic resonances.

Image of FIG. 2.
FIG. 2.

Experimental system for the NO ERE-CARS system.

Image of FIG. 3.
FIG. 3.

Phase-matching geometry employed in the NO ERE-CARS system.

Image of FIG. 4.
FIG. 4.

Polarization arrangement for ERE-CARS detection.

Image of FIG. 5.
FIG. 5.

Experimental NO ERE-CARS spectra demonstrating electronic resonance enhancement at room temperature and subatmospheric pressure for the following conditions (a) and 1% NO, (b) and 1% NO, (c) and NO, and (d) and NO.

Image of FIG. 6.
FIG. 6.

Double-sided Feynman diagrams for the ERE-CARS process corresponding to the following terms in Prior: (Ref. 30) (a) 3, (b) 4, (c) 21, (d) 24, (e) 9, (f) 10, (g) 39, and (h) 42.

Image of FIG. 7.
FIG. 7.

Energy-level diagram of the ERE-CARS process for the ground electronic state of NO.

Image of FIG. 8.
FIG. 8.

Comparison of theoretical (black line) and experimental (red line) ERE-CARS spectra generated for a pressure of , a concentration of NO, and for Raman shifts and Raman transitions of (a) , , (b) , , (c) , , (d) , , (e) , , and (f) , .

Image of FIG. 9.
FIG. 9.

Comparison of theoretical (black line) and experimental (red line) ERE-CARS spectra generated for a pressure of , a concentration of NO, and for Raman shifts and Raman transitions of (a) , , (b) , , and (c) , .

Image of FIG. 10.
FIG. 10.

Enhancement factor for a pressure of , a concentration of NO, and for Raman shifts of (a) , (b) , (c) , (d) , (e) , and (f) .

Image of FIG. 11.
FIG. 11.

Comparison of theoretical (black line) and experimental (red line) ERE-CARS spectra for a pressure of , a concentration of , and probe frequencies of (a) , (b) , and (c) .

Image of FIG. 12.
FIG. 12.

Enhancement factor for a pressure of , a concentration of , and probe frequencies of (a) , (b) , and (c) .

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/content/aip/journal/jcp/128/17/10.1063/1.2909554
2008-05-07
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Perturbative theory and modeling of electronic-resonance-enhanced coherent anti-Stokes Raman scattering spectroscopy of nitric oxide
http://aip.metastore.ingenta.com/content/aip/journal/jcp/128/17/10.1063/1.2909554
10.1063/1.2909554
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