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Coherent control of molecular alignment of homonuclear diatomic molecules by analytically designed laser pulses
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10.1063/1.2976154
/content/aip/journal/jcp/129/12/10.1063/1.2976154
http://aip.metastore.ingenta.com/content/aip/journal/jcp/129/12/10.1063/1.2976154

Figures

Image of FIG. 1.
FIG. 1.

Maximum alignment with the highest rotational state restricted to .

Image of FIG. 2.
FIG. 2.

Rovibrational populations of (a) in the states and under the action of an analytically designed two-photon resonant pulse (b) which is designed to align the at .

Image of FIG. 3.
FIG. 3.

Modulation of frequency of electric field during laser pulse for pulse of 2.5 ps duration [see Eq. (12)].

Image of FIG. 4.
FIG. 4.

Rovibrational populations of (a) in the states , , and under the action of two sequential two-photon resonant pulses (b) which are optimized to align the at .

Tables

Generic image for table
Table I.

Expansion coefficients [see Eq. (18)] for the target states corresponding to maximum alignment when the rotational excitation is restricted to and .

Generic image for table
Table II.

Parameters used for the numerical solution of the TDSE.

Generic image for table
Table III.

Test results arising from the numerical solution of the TDSE for the molecule subject to analytically designed two-photon resonant pulses. The pulses are designed to optimize the alignment of the molecule in its lowest vibrational manifold. Overlaps with optimally aligned wave functions and calculated alignments are shown.

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/content/aip/journal/jcp/129/12/10.1063/1.2976154
2008-09-24
2014-04-23
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Coherent control of molecular alignment of homonuclear diatomic molecules by analytically designed laser pulses
http://aip.metastore.ingenta.com/content/aip/journal/jcp/129/12/10.1063/1.2976154
10.1063/1.2976154
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