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Solute migration caused by excited state absorptions
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View: Figures


Image of FIG. 1.
FIG. 1.

(a) Temporal distributions of an individual pulse (left) and an individual pulse (right). Time originates from the peak of the pulse. (b) The pulse sequence used in this study with a pulse-to-pulse separation of adjustable with respect to . marks the order of each pulse and time refers to the temporal distribution.

Image of FIG. 2.
FIG. 2.

The -scan apparatus used to measure the transmittance (transmitted energy detected by D2 divided by the input optical energy monitored by D1) as a function of the sample position.

Image of FIG. 3.
FIG. 3.

The potential well for the c.m. motion of a solute molecule in the solution.

Image of FIG. 4.
FIG. 4.

The schematic five-energy-band model for ClAlPc. Upward-pointing arrows: optical excitations; wiggly lines: nonradiative relaxations; and downward-pointing arrows: radiative relaxations.

Image of FIG. 5.
FIG. 5.

-scan data of ClAlPc-ethanol obtained with laser pulses. Dots and crosses are for and , respectively.

Image of FIG. 6.
FIG. 6.

-scan data of ClAlPc-ethanol obtained with laser pulses. Dots for , triangles for , crosses for , circles for , and asterisks for .


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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Solute migration caused by excited state absorptions