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Auger recombination and excited state relaxation dynamics in anion clusters
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1.
1.W. U. Huynh, J. J. Dittmer, and A. P. Alivisatos, Science 295, 2425 (2002).
http://dx.doi.org/10.1126/science.1069156
2.
2.V. I. Klimov, A. A. Mikhailovsky, D. W. McBranch, C. A. Leatherdale, and M. G. Bawendi, Science 287, 1011 (2000).
http://dx.doi.org/10.1126/science.287.5455.1011
3.
3.R. D. Schaller, V. M. Agranovich, and V. I. Klimov, Nat. Phys. 1, 189 (2005).
http://dx.doi.org/10.1038/nphys151
4.
4.A. J. Nozik, Chem. Phys. Lett. 457, 3 (2008).
http://dx.doi.org/10.1016/j.cplett.2008.03.094
5.
5.G. Nair, S. M. Geyer, L. Y. Chang, and M. G. Bawendi, Phys. Rev. B 78, 125325 (2008).
http://dx.doi.org/10.1103/PhysRevB.78.125325
6.
6.M. B. Ji, S. Park, S. T. Connor, T. Mokari, Y. Cui, and K. J. Gaffney, Nano Lett. 9, 1217 (2009).
http://dx.doi.org/10.1021/nl900103f
7.
7.A. L. Efros, V. A. Kharchenko, and M. Rosen, Solid State Commun. 93, 301 (1995).
http://dx.doi.org/10.1016/0038-1098(94)00780-2
8.
8.G. Nair and M. G. Bawendi, Phys. Rev. B 76, 081304 (2007).
http://dx.doi.org/10.1103/PhysRevB.76.081304
9.
9.A. Pandey and P. Guyot-Sionnest, J. Chem. Phys. 127, 111104 (2007).
http://dx.doi.org/10.1063/1.2786068
10.
10.P. Guyot-Sionnest, B. Wehrenberg, and D. Yu, J. Chem. Phys. 123, 074709 (2005).
http://dx.doi.org/10.1063/1.2004818
11.
11.A. Pandey and P. Guyot-Sionnest, Science 322, 929 (2008).
http://dx.doi.org/10.1126/science.1159832
12.
12.G. M. Pastor and K. H. Bennemann, in Clusters of Atoms and Molecules, edited by H. Haberland (Springer-Verlag, Berlin, 1994), p. 86.
13.
13.B. Issendorff and O. Cheshnovsky, Annu. Rev. Phys. Chem. 56, 549 (2005).
http://dx.doi.org/10.1146/annurev.physchem.54.011002.103845
14.
14.R. Busani, M. Folkers, and O. Cheshnovsky, Phys. Rev. Lett. 81, 3836 (1998).
http://dx.doi.org/10.1103/PhysRevLett.81.3836
15.
15.R. Busani, R. Giniger, T. Hippler, and O. Cheshnovsky, Phys. Rev. Lett. 90, 083401 (2003).
http://dx.doi.org/10.1103/PhysRevLett.90.083401
16.
16.A. Stolow, A. E. Bragg, and D. M. Neumark, Chem. Rev. (Washington, D.C.) 104, 1719 (2004).
http://dx.doi.org/10.1021/cr020683w
17.
17.G. B. Griffin, A. Kammrath, O. T. Ehrler, R. M. Young, O. Cheshnovsky, and D. M. Neumark, Chem. Phys. 350, 69 (2008).
http://dx.doi.org/10.1016/j.chemphys.2007.12.005
18.
18.A. V. Davis, R. Wester, A. E. Bragg, and D. M. Neumark, J. Chem. Phys. 118, 999 (2003).
http://dx.doi.org/10.1063/1.1536617
19.
19.A. E. Bragg, J. R. R. Verlet, A. Kammrath, O. Cheshnovsky, and D. M. Neumark, J. Chem. Phys. 122, 054314 (2005).
http://dx.doi.org/10.1063/1.1828042
20.
20.J. R. R. Verlet, A. E. Bragg, A. Kammrath, O. Cheshnovsky, and D. M. Neumark, J. Chem. Phys. 121, 10015 (2004).
http://dx.doi.org/10.1063/1.1809573
21.
21.W. C. Wiley and I. H. McLaren, Rev. Sci. Instrum. 26, 1150 (1955).
http://dx.doi.org/10.1063/1.1715212
22.
22.A. T. J. B. Eppink and D. H. Parker, Rev. Sci. Instrum. 68, 3477 (1997).
http://dx.doi.org/10.1063/1.1148310
23.
23.V. Dribinski, A. Ossadtchi, V. A. Mandelshtam, and H. Reisler, Rev. Sci. Instrum. 73, 2634 (2002).
http://dx.doi.org/10.1063/1.1482156
24.
24.U. Hefter, R. D. Mead, P. A. Schulz, and W. C. Lineberger, Phys. Rev. A 28, 1429 (1983).
http://dx.doi.org/10.1103/PhysRevA.28.1429
25.
25.H. Haberland, H. Kornmeier, H. Langosch, M. Oschwald, and G. Tanner, J. Chem. Soc., Faraday Trans. 86, 2473 (1990).
http://dx.doi.org/10.1039/ft9908602473
26.
26.M. E. Garcia, G. M. Pastor, and K. H. Bennemann, Phys. Rev. Lett. 67, 1142 (1991).
http://dx.doi.org/10.1103/PhysRevLett.67.1142
27.
27.H. Kitamura, Eur. Phys. J. D 43, 33 (2007).
http://dx.doi.org/10.1140/epjd/e2007-00069-9
28.
28.C. Brechignac, M. Broyer, P. Cahuzac, G. Delacretaz, P. Labastie, J. P. Wolf, and L. Woste, Phys. Rev. Lett. 60, 275 (1988).
http://dx.doi.org/10.1103/PhysRevLett.60.275
29.
29.S. Leutwyler and J. Bosiger, Chem. Rev. (Washington, D.C.) 90, 489 (1990).
http://dx.doi.org/10.1021/cr00101a004
30.
30.R. S. Berry, J. Chem. Phys. 45, 1228 (1966).
http://dx.doi.org/10.1063/1.1727742
31.
31.N. Gaston, P. Schwerdtfeger, and B. von Issendorff, Phys. Rev. A 74, 043203 (2006).
http://dx.doi.org/10.1103/PhysRevA.74.043203
32.
32.Y. Wang, H. -J. Flad, and M. Dolg, Int. J. Mass Spectrom. 201, 197 (2000).
http://dx.doi.org/10.1016/S1387-3806(00)00157-3
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/content/aip/journal/jcp/130/23/10.1063/1.3149562
2009-06-17
2014-07-25

Abstract

Using femtosecondtime-resolved photoelectron imaging, electron-hole pairs are created in size-selected anion clusters , and the subsequent decay dynamics are measured. These clusters eject electrons via Auger decay on time scales of 100–600 fs. There is an abrupt increase in the Auger decay time for clusters larger than , coinciding with the onset of the transition from van der Waals to covalent bonding in mercury clusters. Our results also show evidence for subpicosecond excited state relaxation attributed to inelastic electron-electron and electron-hole scattering as well as hole-induced contraction of the cluster.

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Scitation: Auger recombination and excited state relaxation dynamics in Hgn−(n=9–20) anion clusters
http://aip.metastore.ingenta.com/content/aip/journal/jcp/130/23/10.1063/1.3149562
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