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Strong fields induce ultrafast rearrangement of H atoms in
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/content/aip/journal/jcp/130/23/10.1063/1.3157234
2009-06-17
2014-09-21

Abstract

H atoms in are rearranged by strong optical fields generated by intense 9.3 fs laser pulses to form . This atomic rearrangement is ultrafast: It occurs within a single laser pulse. Quantum-chemical calculations reveal that originates in the state of when the O–H bond elongates to 1.15 a.u. and the H–O–H angle becomes 120°. Bond formation on the ultrafast time scale of molecular vibrations (10 fs for ) and in strong fields has hitherto not been reported.

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Scitation: Strong fields induce ultrafast rearrangement of H atoms in H2O
http://aip.metastore.ingenta.com/content/aip/journal/jcp/130/23/10.1063/1.3157234
10.1063/1.3157234
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