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Quantum control study of multilevel effect on ultrafast isotope-selective vibrational excitations
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10.1063/1.3245401
/content/aip/journal/jcp/131/14/10.1063/1.3245401
http://aip.metastore.ingenta.com/content/aip/journal/jcp/131/14/10.1063/1.3245401

Figures

Image of FIG. 1.
FIG. 1.

The OCT results within the density-matrix formalism for case (A1) . (a) The optimal control field . (b) The spectrum of the optimal field. (c) Temporal change in the populations of vibrational eigenstates for . (d) That for .

Image of FIG. 2.
FIG. 2.

The OCT results within the density-matrix formalism for case (A2) . [(a)–(d)] The same as in Fig. 1.

Image of FIG. 3.
FIG. 3.

Temporal changes in the phase of wave packet for (black) and (red) in the four periods of time: ; ; ;

Image of FIG. 4.
FIG. 4.

The OCT results within the density-matrix formalism for case (A3) . [(a)–(d)] The same as in Fig. 1.

Image of FIG. 5.
FIG. 5.

The OCT results within the density-matrix formalism for case (A6) . [(a)–(d)] The same as in Fig. 1.

Image of FIG. 6.
FIG. 6.

The OCT results within the wave-packet formalism for case (B1) . [(a)–(d)] The same as in Fig. 1. (e) The time propagations of the wave packets for (black) and (red).

Image of FIG. 7.
FIG. 7.

The OCT results within the wave-packet formalism for case (B2) . [(a)–(e)] The same as in Fig. 6.

Tables

Generic image for table
Table I.

Energies of the lowest 10 vibrational eigenstates of the PECs for and relative to the PEC bottom .

Generic image for table
Table II.

Sets of total time and the number of basis functions considered in the present OCT calculations and the maximum field amplitudes and the yields for the resultant optimal electric fields.

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/content/aip/journal/jcp/131/14/10.1063/1.3245401
2009-10-12
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Quantum control study of multilevel effect on ultrafast isotope-selective vibrational excitations
http://aip.metastore.ingenta.com/content/aip/journal/jcp/131/14/10.1063/1.3245401
10.1063/1.3245401
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