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Tracing ultrafast hydrogen migration in allene in intense laser fields by triple-ion coincidence momentum imaging
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Image of FIG. 1.

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FIG. 1.

Schematic diagrams of the two angle parameters, and , and the correlation maps for the pathways of (a) and (b) .

Image of FIG. 2.

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FIG. 2.

The geometrical structure of constructed from the observed momentum vectors of the respective fragment ions ejected through the Coulomb explosion of pathway (1), (left), and pathway (2), (right). The two red horizontal bars represent the ranges of the position of the charge centers of the two heavy moieties.

Image of FIG. 3.

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FIG. 3.

(a) The distributions for pathway (1) and pathway (2) and (b) schematic diagram of the parent allene molecule for forming the precursor species, and , by the extent of the proton migration.

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/content/aip/journal/jcp/131/15/10.1063/1.3251032
2009-10-16
2014-04-16

Abstract

Ultrafast hydrogen migration in allene in intense laser fields was investigated by triple-ion coincidence momentum imaging. The migrating proton covering the entire range of an allene molecule was visualized by the momentum correlation maps and by the geometrical structure of triply charged allene reconstructed from the observed momentum vectors of fragment ions. The extent of hydrogen migration was found to play a decisive role in breaking selectively one of the two initially equivalent C–C chemical bonds that become inequivalent in the course of the hydrogen migration.

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Scitation: Tracing ultrafast hydrogen migration in allene in intense laser fields by triple-ion coincidence momentum imaging
http://aip.metastore.ingenta.com/content/aip/journal/jcp/131/15/10.1063/1.3251032
10.1063/1.3251032
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