1887
banner image
No data available.
Please log in to see this content.
You have no subscription access to this content.
No metrics data to plot.
The attempt to load metrics for this article has failed.
The attempt to plot a graph for these metrics has failed.
The full text of this article is not currently available.
f
Vibrational spectroscopy of neutral silicon clusters via far-IR-VUV two color ionization
Rent:
Rent this article for
Access full text Article
/content/aip/journal/jcp/131/17/10.1063/1.3262803
1.
1.U. Röthlisberger, W. Andreoni, and M. Parrinello, Phys. Rev. Lett. 72, 665 (1994).
http://dx.doi.org/10.1103/PhysRevLett.72.665
2.
2.A. Tekin and B. Hartke, J. Theor. Comput. Chem. 4, 1119 (2005).
http://dx.doi.org/10.1142/S0219633605002008
3.
3.S. Goedecker, W. Hellmann, and T. Lenosky, Phys. Rev. Lett. 95, 055501 (2005).
http://dx.doi.org/10.1103/PhysRevLett.95.055501
4.
4.E. C. Honea, A. Ogura, C. A. Murray, K. Raghavachari, W. O. Sprenger, M. F. Jarrold, and W. L. Brown, Nature (London) 366, 42 (1993).
http://dx.doi.org/10.1038/366042a0
5.
5.E. C. Honea, A. Ogura, D. R. Peale, C. Felix, C. A. Murray, K. Raghavachari, W. O. Sprenger, M. F. Jarrold, and W. L. Brown, J. Chem. Phys. 110, 12161 (1999).
http://dx.doi.org/10.1063/1.479153
6.
6.S. Li, R. J. Van Zee, J. W. Weltner, and K. Raghavachari, Chem. Phys. Lett. 243, 275 (1995).
http://dx.doi.org/10.1016/0009-2614(95)00836-S
7.
7.K. Fuke, K. Tsukamoto, F. Misaizu, and M. Sanekata, J. Chem. Phys. 99, 7807 (1993).
http://dx.doi.org/10.1063/1.465658
8.
8.K. D. Rinnen and M. L. Mandich, Phys. Rev. Lett. 69, 1823 (1992).
http://dx.doi.org/10.1103/PhysRevLett.69.1823
9.
9.G. Meloni and K. A. Gingerich, J. Chem. Phys. 115, 5470 (2001).
http://dx.doi.org/10.1063/1.1391265
10.
10.K. -M. Ho, A. A. Shvartsburg, B. Pan, Z. -Y. Lu, C. -Z. Wang, J. G. Wacker, J. L. Fye, and M. F. Jarrold, Nature (London) 392, 582 (1998).
http://dx.doi.org/10.1038/33369
11.
11.A. A. Shvartsburg, R. R. Hudgins, P. Dugourd, and M. F. Jarrold, Chem. Soc. Rev. 30, 26 (2001).
http://dx.doi.org/10.1039/a802099j
12.
12.O. Cheshnovsky, S. H. Yang, C. L. Pettiette, M. J. Craycraft, Y. Liu, and R. E. Smalley, Chem. Phys. Lett. 138, 119 (1987).
http://dx.doi.org/10.1016/0009-2614(87)80353-6
13.
13.J. Müller, B. Liu, A. A. Shvartsburg, S. Ogut, J. R. Chelikowsky, K. W. M. Siu, K. -M. Ho, and G. Gantefor, Phys. Rev. Lett. 85, 1666 (2000).
http://dx.doi.org/10.1103/PhysRevLett.85.1666
14.
14.M. Astruc Hoffmann, G. Wrigge, B. v. Issendorff, J. Müller, G. Ganteför, and H. Haberland, Eur. Phys. J. D 16, 9 (2001).
http://dx.doi.org/10.1007/s100530170048
15.
15.G. Meloni, M. J. Ferguson, S. M. Sheehan, and D. M. Neumark, Chem. Phys. Lett. 399, 389 (2004).
http://dx.doi.org/10.1016/j.cplett.2004.10.030
16.
16.J. Bai, L. -F. Cui, J. Wang, S. Yoo, X. Li, J. Jellinek, C. Koehler, T. Frauenheim, L. -S. Wang, and X. C. Zeng, J. Phys. Chem. A 110, 908 (2006).
http://dx.doi.org/10.1021/jp055874s
17.
17.T. N. Kitsopoulos, C. J. Chick, A. Weaver, and D. M. Neumark, J. Chem. Phys. 93, 6108 (1990).
http://dx.doi.org/10.1063/1.459004
18.
18.G. S. Icking-Konert, H. Handschuh, P. S. Bechthold, G. Ganteför, B. Kessler, and W. Eberhardt, Surf. Rev. Lett. 3, 483 (1996).
http://dx.doi.org/10.1142/S0218625X96000875
19.
19.C. Xu, T. R. Taylor, G. R. Burton, and D. M. Neumark, J. Chem. Phys. 108, 1395 (1998).
http://dx.doi.org/10.1063/1.475511
20.
20.J. T. Lyon, P. Gruene, A. Fielicke, G. Meijer, E. Janssens, P. Claes, and P. Lievens, J. Am. Chem. Soc. 131, 1115 (2009).
http://dx.doi.org/10.1021/ja807518y
21.
21.P. Gruene, A. Fielicke, G. Meijer, E. Janssens, V. T. Ngan, M. T. Nguyen, and P. Lievens, ChemPhysChem 9, 703 (2008).
http://dx.doi.org/10.1002/cphc.200800015
22.
22.K. R. Asmis, A. Fielicke, G. von Helden, and G. Meijer, in Atomic Clusters: From Gas Phase to Deposited, edited by D. P. Woodruff (Elsevier, Amsterdam, 2007), p. 327.
23.
23.M. B. Knickelbein, J. Chem. Phys. 100, 4729 (1994).
http://dx.doi.org/10.1063/1.466263
24.
24.R. Gehrke, P. Gruene, A. Fielicke, G. Meijer, and K. Reuter, J. Chem. Phys. 130, 034306 (2009).
http://dx.doi.org/10.1063/1.3058637
25.
25.K. R. Asmis and J. Sauer, Mass Spectrom. Rev. 26, 542 (2007).
http://dx.doi.org/10.1002/mas.20136
26.
26.P. Gruene, D. M. Rayner, B. Redlich, A. F. G. van der Meer, J. T. Lyon, G. Meijer, and A. Fielicke, Science 321, 674 (2008).
http://dx.doi.org/10.1126/science.1161166
27.
27.G. von Helden, I. Holleman, G. M. H. Knippels, A. F. G. van der Meer, and G. Meijer, Phys. Rev. Lett. 79, 5234 (1997).
http://dx.doi.org/10.1103/PhysRevLett.79.5234
28.
28.G. von Helden, D. van Heijnsbergen, and G. Meijer, J. Phys. Chem. A 107, 1671 (2003).
http://dx.doi.org/10.1021/jp021982s
29.
29.M. Putter, G. von Helden, and G. Meijer, Chem. Phys. Lett. 258, 118 (1996).
http://dx.doi.org/10.1016/0009-2614(96)00656-2
30.
30.W. Bouwen, P. Thoen, F. Vanhoutte, S. Bouckaert, F. Despa, H. Weidele, R. E. Silverans, and P. Lievens, Rev. Sci. Instrum. 71, 54 (2000).
http://dx.doi.org/10.1063/1.1150159
31.
31.D. J. Trevor, D. M. Cox, K. C. Reichmann, R. O. Brickman, and A. Kaldor, J. Phys. Chem. 91, 2598 (1987).
http://dx.doi.org/10.1021/j100294a030
32.
32.D. Oepts, A. F. G. van der Meer, and P. W. van Amersfoort, Infrared Phys. Technol. 36, 297 (1995).
http://dx.doi.org/10.1016/1350-4495(94)00074-U
33.
33.M. J. Frisch, G. W. Trucks, H. B. Schlegel et al., GAUSSIAN 03, Revision C.02, Gaussian, Inc., Wallingford, CT, 2004.
34.
34.See EPAPS supplementary material at http://dx.doi.org/10.1063/1.3262803 for details of the quantum chemical calculations.[Supplementary Material]
35.
35.C. Zhao and K. Balasubramanian, J. Chem. Phys. 116, 3690 (2002).
http://dx.doi.org/10.1063/1.1446027
36.
36.A. D. Zdetsis, J. Chem. Phys. 127, 014314 (2007).
http://dx.doi.org/10.1063/1.2746030
37.
37.P. Karamanis, D. Zhang-Negrerie, and C. Pouchan, Chem. Phys. 331, 417 (2007).
http://dx.doi.org/10.1016/j.chemphys.2006.11.013
38.
38.K. Raghavachari and C. M. Rohlfing, Chem. Phys. Lett. 198, 521 (1992).
http://dx.doi.org/10.1016/0009-2614(92)80038-D
39.
39.X. Zhu and X. C. Zeng, J. Chem. Phys. 118, 3558 (2003).
http://dx.doi.org/10.1063/1.1535906
http://aip.metastore.ingenta.com/content/aip/journal/jcp/131/17/10.1063/1.3262803
Loading
/content/aip/journal/jcp/131/17/10.1063/1.3262803
Loading

Data & Media loading...

Loading

Article metrics loading...

/content/aip/journal/jcp/131/17/10.1063/1.3262803
2009-11-05
2014-11-28

Abstract

Tunable far-infrared-vacuum-ultraviolet two color ionization is used to obtain vibrational spectra of neutral silicon clusters in the gas phase. Upon excitation with tunable infrared light prior to irradiation with UVphotons we observe strong enhancements in the mass spectrometric signal of specific cluster sizes. This allowed the recording of the infrared absorption spectra of , , and . Structural assignments were made by comparison with calculated linear absorption spectra from quantum chemical theory.

Loading

Full text loading...

/deliver/fulltext/aip/journal/jcp/131/17/1.3262803.html;jsessionid=60ugfnn0tjsml.x-aip-live-02?itemId=/content/aip/journal/jcp/131/17/10.1063/1.3262803&mimeType=html&fmt=ahah&containerItemId=content/aip/journal/jcp
true
true
This is a required field
Please enter a valid email address
752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Vibrational spectroscopy of neutral silicon clusters via far-IR-VUV two color ionization
http://aip.metastore.ingenta.com/content/aip/journal/jcp/131/17/10.1063/1.3262803
10.1063/1.3262803
SEARCH_EXPAND_ITEM