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Study of the ground multiplet of Kramers rare earth ions in solid matrices by multifrequency electron paramagnetic resonance spectroscopy: in single-crystals
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10.1063/1.3180697
/content/aip/journal/jcp/131/3/10.1063/1.3180697
http://aip.metastore.ingenta.com/content/aip/journal/jcp/131/3/10.1063/1.3180697

Figures

Image of FIG. 1.
FIG. 1.

The parallel EPR transitions of in PWO at 10 K. The experimental (upper line) and the simulated (lower line) spectra obtained at 9.43 GHz (a), 95 GHz (b), and 190 GHz (c), respectively.

Image of FIG. 2.
FIG. 2.

The perpendicular HF-EPR spectra of in PWO at 10 K. The experimental (upper line) and the simulated (lower line) spectra obtained at 95 GHz.

Image of FIG. 3.
FIG. 3.

The calculated (with the parameters given in Table II) HF effect at 285 GHz on the line position at the perpendicular orientation and the corresponding experimental data at , 20°, 25°, and 45°.

Image of FIG. 4.
FIG. 4.

Energy-level diagram of the ground multiplet in PWO for the orientations -axis as a function of the magnetic field. The length of the vertical line corresponds to the 190 GHz radiation energy and the line position marks the EPR transition. The energy levels at zero magnetic field are listed in Table III.

Image of FIG. 5.
FIG. 5.

Energy-level diagram of the in PWO for the orientation -axis as a function of the magnetic field. The length of the vertical line corresponds to the 285 GHz radiation energy and the line position marks the EPR transition. The energy levels at zero magnetic field are listed in Table III.

Tables

Generic image for table
Table I.

The parameters of the axial spin Hamiltonian of in PWO single crystals measured at for several frequencies, determined with Eq. (1) and . The values are given in units.

Generic image for table
Table II.

The parameter values of the Hamiltonian [see Eqs. (6) and (7)]. All the values are .

Generic image for table
Table III.

The experimental data for in PWO measured by optical (from Ref. 9) and EPR spectroscopy. The corresponding calculated data are also presented.

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/content/aip/journal/jcp/131/3/10.1063/1.3180697
2009-07-17
2014-04-19
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Study of the ground multiplet of Kramers rare earth ions in solid matrices by multifrequency electron paramagnetic resonance spectroscopy: Nd3+ in PbWO4 single-crystals
http://aip.metastore.ingenta.com/content/aip/journal/jcp/131/3/10.1063/1.3180697
10.1063/1.3180697
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