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Field-free molecular orientation with terahertz few-cycle pulses
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10.1063/1.3458913
/content/aip/journal/jcp/132/24/10.1063/1.3458913
http://aip.metastore.ingenta.com/content/aip/journal/jcp/132/24/10.1063/1.3458913

Figures

Image of FIG. 1.
FIG. 1.

(a) Electric field (solid line) used for the exact TDSE and RRA calculations, and kicked field (dashed lines) consisting of seven consecutive kicks used for the IA. (b) Fourier transforms of pulse in frequency domain. , , , , , , and .

Image of FIG. 2.
FIG. 2.

The evolution of the degree of orientation for LiH by using the three levels of approximations, where the rotational temperature is .

Image of FIG. 3.
FIG. 3.

The final rotational populations calculated by the RRA and the IA for LiH.

Image of FIG. 4.
FIG. 4.

The evolution of the degree of orientation for LiCl as a function of laser frequency , where the intensity of electric fields are and , and the other pulse parameters are the same as those in Fig. 1.

Image of FIG. 5.
FIG. 5.

The evolutions of the degree of orientation obtained by using the exact TDSE calculation and the RRA for LiCl.

Image of FIG. 6.
FIG. 6.

Time-dependent rotational populations of in the vibrational state for LiCl.

Image of FIG. 7.
FIG. 7.

The evolutions of the degree of orientation calculated by using the RRA and the IA for LiCl. The letter marks indicate the short instants.

Image of FIG. 8.
FIG. 8.

Polar plots of angular distributions at different times marked in Fig. 7 for LiCl.

Tables

Generic image for table
Table I.

Molecular parameters.

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/content/aip/journal/jcp/132/24/10.1063/1.3458913
2010-06-28
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Field-free molecular orientation with terahertz few-cycle pulses
http://aip.metastore.ingenta.com/content/aip/journal/jcp/132/24/10.1063/1.3458913
10.1063/1.3458913
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