1887
banner image
No data available.
Please log in to see this content.
You have no subscription access to this content.
No metrics data to plot.
The attempt to load metrics for this article has failed.
The attempt to plot a graph for these metrics has failed.
Biexponential theory of Drude dissipation via hierarchical quantum master equation
Rent:
Rent this article for
USD
10.1063/1.3491270
/content/aip/journal/jcp/133/11/10.1063/1.3491270
http://aip.metastore.ingenta.com/content/aip/journal/jcp/133/11/10.1063/1.3491270
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

vs at some selected values of .

Image of FIG. 2.
FIG. 2.

(a) and (b) as functions of [cf. Eqs. (12) and (13), respectively].

Image of FIG. 3.
FIG. 3.

Density matrix evolutions: exact (red line), HQME0 (gray dashed line), and HQME1 (black line). The energy parameters are reported in units of , while the time variable is in units of . Both the applicability parameters, and , are about equal to or larger than 5 [cf. Eq. (15a)].

Image of FIG. 4.
FIG. 4.

The same as in Fig. 3, but with one applicability parameter, , being around the boundary of applicability [cf. Eq. (15b)].

Image of FIG. 5.
FIG. 5.

The same as in Fig. 3, but with the applicability parameters, and , being both around the boundary of applicability [cf. Eq. (15b)].

Image of FIG. 6.
FIG. 6.

Transient absorption signals via HQME1 (black line) vs the exact dynamics (thin red line) of the model dimer exciton system (see parameters in text) at . This is in the HQME1 accurate regime by Eq. (15a); i.e., both and are larger than 5. (a) Linear absorption coefficient , (b) nonlinear absorptive , and (c) nonlinear emissive components of the frequency-dispersed difference transient probe absorption coefficient. The pump pulse frequency is centered at , as indicated by the arrow in panel (a).

Image of FIG. 7.
FIG. 7.

The same as in Fig. 6, but now the system is at , falling into the HQME1 semiquantitative regime by Eq. (15b).

Loading

Article metrics loading...

/content/aip/journal/jcp/133/11/10.1063/1.3491270
2010-09-21
2014-04-17
Loading

Full text loading...

This is a required field
Please enter a valid email address
752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Biexponential theory of Drude dissipation via hierarchical quantum master equation
http://aip.metastore.ingenta.com/content/aip/journal/jcp/133/11/10.1063/1.3491270
10.1063/1.3491270
SEARCH_EXPAND_ITEM