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Absolute measurement of the S(0) and S(1) lines in the electric quadrupole fundamental band of around
1.B. P. Lanyon, J. D. Whitfield, G. G. Gillett, M. E. Goggin, M. P. Almeida, I. Kassal, J. D. Biamonte, M. Mohseni, B. J. Powell, M. Barbieri, A. Aspuru-Guzik, and A. G. White, Nat. Chem. 2, 106 (2010).
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The electric quadrupole fundamental band of molecular deuterium around is accessed by cavity ring-down spectroscopy using a difference-frequency-generation source linked to the Cs-clock primary standard via an optical frequency combsynthesizer. An absolute determination of the line position and strength is reported for the first two transitions ( and ) of the S branch. An accuracy of is achieved for the line-center frequencies, which improves by a factor 20 previous experimental results [A. R. W. McKellar and T. Oka, Can. J. Phys.56, 1315 (1978)]. The line strength values, measured with 1% accuracy, are used to retrieve the quadrupole moment matrix elements which are found in good agreement with previous theoretical calculations [A. Birnbaum and J. D. Poll, J. Atmos. Sci.26, 943 (1969); J. L. Hunt, J. D. Poll, and L. Wolniewicz, Can. J. Phys.62, 1719 (1984)].
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