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Absolute measurement of the S(0) and S(1) lines in the electric quadrupole fundamental band of around
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/content/aip/journal/jcp/133/15/10.1063/1.3493393
2010-10-21
2014-10-25

Abstract

The electric quadrupole fundamental band of molecular deuterium around is accessed by cavity ring-down spectroscopy using a difference-frequency-generation source linked to the Cs-clock primary standard via an optical frequency combsynthesizer. An absolute determination of the line position and strength is reported for the first two transitions ( and ) of the S branch. An accuracy of is achieved for the line-center frequencies, which improves by a factor 20 previous experimental results [A. R. W. McKellar and T. Oka, Can. J. Phys.56, 1315 (1978)]. The line strength values, measured with 1% accuracy, are used to retrieve the quadrupole moment matrix elements which are found in good agreement with previous theoretical calculations [A. Birnbaum and J. D. Poll, J. Atmos. Sci.26, 943 (1969); J. L. Hunt, J. D. Poll, and L. Wolniewicz, Can. J. Phys.62, 1719 (1984)].

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Scitation: Absolute measurement of the S(0) and S(1) lines in the electric quadrupole fundamental band of D2 around 3 μm
http://aip.metastore.ingenta.com/content/aip/journal/jcp/133/15/10.1063/1.3493393
10.1063/1.3493393
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