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Polarization of molecular targets using infrared stimulated Raman adiabatic passage
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10.1063/1.3475523
/content/aip/journal/jcp/133/9/10.1063/1.3475523
http://aip.metastore.ingenta.com/content/aip/journal/jcp/133/9/10.1063/1.3475523

Figures

Image of FIG. 1.
FIG. 1.

S(2) transition with two resonant -polarized photons.

Image of FIG. 2.
FIG. 2.

S(2) transition with biaxial excitation, i.e., combined - and -polarized photons. The blue arrows represent -polarized photons and red and yellow arrows represent - and -polarized photons, respectively.

Image of FIG. 3.
FIG. 3.

Interaction diagram showing four interfering pathways to generate the optical coherence . For details, see Ref. 18.

Image of FIG. 4.
FIG. 4.

Interaction diagrams showing four interfering pathways generating the optical coherence . For details, see Ref. 18.

Image of FIG. 5.
FIG. 5.

Nearly complete population transfer to the level using IR STIRAP with the counterintuitive sequence of Gaussian pulses of duration and interpulse delay of for (a) with Rabi frequency , laser intensity , and population transfer of 100%; (b) with Rabi frequency , laser intensity , and population transfer of 94%; and (c) with Rabi frequency , laser intensity , and population transfer of 92%.

Image of FIG. 6.
FIG. 6.

Zeeman population distribution in the final level using IR STIRAP at the end of excitation with the counterintuitive sequence of Gaussian pulses of duration and interpulse delay of : (a) ; (b) ; and (c) . Rabi frequencies and laser power for each transition are the same as in Fig. 5.

Image of FIG. 7.
FIG. 7.

Three-dimensional polar plot of the angular momentum polarization in the final level using IR STIRAP with the counterintuitive sequence of Gaussian pulses for (a) with alignment parameters and ; (b) with alignment parameters and ; and (c) with alignment parameters and . The pulse duration, delay, and laser power are identical to those of Figs. 5 and 6.

Tables

Generic image for table
Table I.

Definitions of the terms found in Eqs. (7)–(16).

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/content/aip/journal/jcp/133/9/10.1063/1.3475523
2010-09-02
2014-04-21
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Polarization of molecular targets using infrared stimulated Raman adiabatic passage
http://aip.metastore.ingenta.com/content/aip/journal/jcp/133/9/10.1063/1.3475523
10.1063/1.3475523
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