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/content/aip/journal/jcp/134/24/10.1063/1.3608061
2011-06-24
2016-08-30

Abstract

A 1 + 1multiphoton ionization (MPI) detection scheme for OH radicals is presented. The spectroscopic approach combines initial excitation on the well-characterized A2Σ+–X2Π band system with vacuum ultraviolet (VUV)ionization via autoionizing Rydberg states that converge on the OH+ A3Π ion state. Jet-cooled MPI spectra on the (1,0) and (2,0) bands show anomalous rotational line intensities, while initial excitation on the (0,0) band does not lead to detectable OH+ ions. The onset of ionization with the (1,0) band is attributed to an energetic threshold; the combined UV + VUVphoton energies are above the first member of the autoionizing (A3Π)nd Rydberg series. Comparison of the OH 1 + 1 MPI signal with that from single photonVUVionization of NO indicates that the cross section for photoionization from OH A2Σ+, v = 1 is on the order of 10−17 cm2.

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