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/content/aip/journal/jcp/134/3/10.1063/1.3533274
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/content/aip/journal/jcp/134/3/10.1063/1.3533274
2011-01-19
2016-12-06

Abstract

The optical Stark spectrum of the E(0+) − X 1Σ+ (1,0) band of thorium monoxide, ThO, was recorded and analyzed to determine the permanent electric dipole moments,μ, for the E(0+) (v = 1) and X 1Σ+ (v = 0) states. Values of 2.782 ± 0.012 D (X) and 3.534 ± 0.010 D (E) were obtained. The uncertainties are 2σ statistical error. The systematic errors are estimated to be less than 1%. The experimental results are used to access the quality of electronic structure calculations of the properties of the X 1Σ+ (v = 0) state.

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