Schematic illustration of the experimental setup.
Angular dependent strong field ionization yield of sulfur atom produced from photodissociation of (a) ethylene sulfide (b) carbonyl sulfide at 193 nm. The red curves are the fitted results (see fitting method in the main text).
Basis functions: the angular dependent ionization probabilities.
Extracted |m l | distributions of sulfur atom (1D2) from photodissociation of (a) ethylene sulfide (b) carbonyl sulfide. The right portion of each figure is the constructed electron charge cloud of the sulfur atom showing small degree of alignment along the pump laser polarization.
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